The bore on the 427 is larger than that of an LS3/6.2
4.125" on the
427
4.065" on the
LS3
As car as I can tell, the stroke is the same at 3.622"
So you
could put a longer rod / shorter stroke rotating assembly in the 427 to possibly get down to 6.2L but it would be a different bore/stroke ratio than an LS3. This would very likely need to be a custom crankshaft unless by some coincidence one of the other LS family cranks magically results in a 6.2L with a 4.125" bore.